Disc 1

1. "Bleecker Street" (Demo)
2. "The Sound of Silence"
3. "The Sun Is Burning"
4. "Wednesday Morning, 3 AM"
5. "He Was My Brother"
6. "Sparrow"
7. "Peggy-O"
8. "Benedictus"
9. "Somewhere They Can't Find Me"
10. "We've Got a Groovy Thing Goin'"
11. "Leaves That Are Green"
12. "Richard Cory"
13. "I Am a Rock"
14. "The Sound of Silence" (Single Version)
15. "Homeward Bound"
16. "Blues Runs the Game"
17. "Kathy's Song"
18. "April Come She Will"
19. "Flowers Never Bend with the Rainfall"

Disc 2

1. "Patterns"
2. "Cloudy"
3. "The Dangling Conversation"
4. "Scarborough Fair/Canticle"
5. "The 59th Street Bridge Song (Feelin' Groovy)"
6. "For Emily, Whenever I May Find Her"
7. "7 O'Clock News/Silent Night"
8. "A Hazy Shade of Winter"
9. "At the Zoo"
10. "A Poem on the Underground Wall" (Live)
11. "Red Rubber Ball" (Live in New York City, 1967) - appears only on this collection
12. "Blessed" (Live)
13. "Anji" (Live)
14. "A Church Is Burning" (Live)
15. "Fakin' It"
16. "Save the Life of My Child"
17. "America"
18. "You Don't Know Where Your Interest Lies"
19. "Punky's Dilemma"
20. "Comfort and Joy" - appears only on this collection
21. "Star Carol" - appears only on this collection

Disc 3

1. "Mrs. Robinson"
2. "Old Friends/Bookends"
3. "Overs"
4. "A Most Peculiar Man" (Live)
5. "Bye, Bye Love" (Live)
6. "The Boxer"
7. "Baby Driver"
8. "Why Don't You Write Me"
9. "Feuilles-O" (Demo)
10. "Keep the Customer Satisfied"
11. "So Long, Frank Lloyd Wright"
12. "Song for the Asking"
13. "Cecilia"
14. "El Condor Pasa (If I Could)"
15. "Bridge Over Troubled Water"
16. "The Only Living Boy In New York"
17. "Hey, Schoolgirl/Black Slacks" (Live)
18. "That Silver Haired Daddy of Mine" (Live)
19. "My Little Town"